Atmospheric Tomography: A Bayesian inversion technique for determining the rate and location of fugitive emissions

A Bayesian inversion technique to determine the location and strength of trace gas emissions from a point source in open air is presented. It was tested using atmospheric measurements of nitrous oxide (N2O) and carbon dioxide (CO2) released at known rates from a source located within an array of eight evenly spaced sampling points on a 20 m radius circle. The analysis requires knowledge of concentration enhancement downwind of the source and the normalized, three-dimensional distribution (shape) of concentration in the dispersion plume. The influence of varying background concentrations of ~1% for N2O and ~10% for CO2 was removed by subtracting upwind concentrations from those downwind of the source to yield only concentration enhancements. Continuous measurements of turbulent wind and temperature statistics were used to model the dispersion plume. The analysis localized the source to within 0.8 m of the true position and the emission rates were determined to better than 3% accuracy. This technique will be useful in assurance monitoring for geological storage of CO2 and for applications requiring knowledge of the location and rate of fugitive emissions.

Simple

Identification info

Date (Publication)
2011-01-01T00:00:00
Citation identifier
Geoscience Australia Persistent Identifier/https://pid.geoscience.gov.au/dataset/ga/72702

Citation identifier
Digital Object Identifier/http://dx.doi.org/10.1021/es202807s

Cited responsible party
Role Organisation / Individual Name Details
Author

Humphries, R.

 1
Author

Jenkins, C.

 2
Author

Leuning, R.

 3
Author

Zegelin, S.

 4
Author

Griffith, D.

 5
Author

Caldow, C.

 6
Author

Berko, H.

 7
Author

Feitz, A.J.

 8
ISBN

0013-936X

Point of contact
Role Organisation / Individual Name Details
Custodian

ED
Owner

Commonwealth of Australia (Geoscience Australia)
Custodian

Commonwealth of Australia (Geoscience Australia)

 Voice
Topic category
  • Geoscientific information

Extent

N
S
E
W


Maintenance and update frequency
Unknown

Resource format

Title

Product data repository: Various Formats

Protocol

FILE:DATA-DIRECTORY

Name of the resource

Data Store directory containing the digital product files

Description

Data Store directory containing one or more files, possibly in a variety of formats, accessible to Geoscience Australia staff only for internal purposes

Keywords

  • External Publication

  • Scientific Journal Paper

Theme

  • carbon dioxide

  • geological storage of CO2

  • geological sequestration

  • greenhouse gas emissions

  • model

Keywords

  • AU-ACT

Australian and New Zealand Standard Research Classification (ANZSRC)

  • Earth Sciences

Keywords

  • Published_External

Resource constraints

Title

Creative Commons Attribution 4.0 International Licence

Alternate title

CC-BY

Edition

4.0

Website

http://creativecommons.org/licenses/

Access constraints
License
Use constraints
License

Resource constraints

Title

Australian Government Security ClassificationSystem

Edition date
2018-11-01T00:00:00
Website

https://www.protectivesecurity.gov.au/Pages/default.aspx

Classification
Unclassified
Language
English
Character encoding
UTF8

Distribution Information

Distributor contact
Role Organisation / Individual Name Details
Distributor

Commonwealth of Australia (Geoscience Australia)

 Voice
OnLine resource

Link to Publication

Link to Publication

Resource lineage

Statement

Unknown

Hierarchy level
Non geographic dataset
Other

External Publication

Description

Source data not available.

Metadata constraints

Title

Australian Government Security ClassificationSystem

Edition date
2018-11-01T00:00:00
Website

https://www.protectivesecurity.gov.au/Pages/default.aspx

Classification
Unclassified

Metadata

Metadata identifier
urn:uuid/a968033f-e72e-5b4b-e044-00144fdd4fa6

Title

GeoNetwork UUID

Language
English
Character encoding
UTF8
Contact
Role Organisation / Individual Name Details
Point of contact

Commonwealth of Australia (Geoscience Australia)

 Voice

Type of resource

Resource scope
Document
Name

nonGeographicDataset

Alternative metadata reference

Title

Geoscience Australia - short identifier for metadata record with

uuid

Citation identifier
eCatId/72702

Metadata linkage

https://ecat.ga.gov.au/geonetwork/srv/eng/catalog.search#/metadata/a968033f-e72e-5b4b-e044-00144fdd4fa6

Date info (Revision)
2018-04-20T06:11:45
Date info (Creation)
2011-08-01T00:00:00

Metadata standard

Title

AU/NZS ISO 19115-1:2014

Metadata standard

Title

ISO 19115-1:2014

Metadata standard

Title

ISO 19115-3

Title

Geoscience Australia Community Metadata Profile of ISO 19115-1:2014

Edition

Version 2.0, September 2018

Citation identifier
https://pid.geoscience.gov.au/dataset/ga/122551

 
 

Spatial extent

N
S
E
W


Keywords

carbon dioxide geological sequestration geological storage of CO2 greenhouse gas emissions model

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